You will probably be better off creating your own device DTS.
I think the first file is 'the right one', although you must also include the serial.ko (I think that's what it is called) in the image also. This can be included when you create your own device definition in the .mk file. You could copy/paste any other similar device. ( Look at the .mk files and see what other devices include, in terms of .ko files. )
Then enable UART as above, then include the serial.ko or appropriate driver for UART usage.
You don't need to touch .dtsi, all the changes should be made in the specific device file.
Both uartlite2 and uartlite3 are defined in mt7621.dtsi but they are disabled there. What you need to do is enable them in your device specific .dts
Then in mt7621_unielec_u7621-06.dtsi "uart2" is included into gpio list, so in your device specific .dts you need to mimic this section but with uart2 excluded.