That is not a supported operation, unmodified OpenWrt will not work on such devices and it's a pretty risky operation.
In short, you'd have to change the partitioning, adapt the bootloader to search in the right place (this probably requires recompiling it), move partitions around, modify the NAND partitions in the DTS, change the sysupgrade support, image generation and half a dozen other places (which you will have to keep rebasing/ rebuilding till the dawn of time). It can be done, but it's very risky - and if you have to ask about anything, you can't do it.